Pattern formation in photorefractive media

Schematic pattern forming experiment
Schematic experimental setup: a homogeneous pump beam interacts nonlinearily with a second pump beam obtained by reflection at an exteral mirror. Interplay of nonequilibrium system, nonlinearity and spatial coupling by means of the single-mirror feedback results in the spontaneous generation of selforganized transverse patterns across beam.
Two counterpropagating laser beams interacting in a photorefractive medium display self-organized generation of spatial patterns. The photorefractive two-wave mixing nonlinearity is mediated by the self-induced generation of a longitudinal refractive index grating - a Bragg mirror - as a result of the pump beam interference. The second pump beam is obtained by a reflection off an external feedback mirror. As is usual in pattern forming systems, one can identifiy two antagonistic processes: on one hand the generation of the self-induced Bragg mirror, on the other hand the pump beam depletion caused by the Bragg mirror which thereby depletes its own source. The solution of this antagonism is the spatial structuring of the system: Regions with low Bragg mirror amplitude provide high transmission of the incident pump beam. The transmitted parts of the pump beam propagate to the external mirror and back and created regions with a high Bragg mirror amplitude.
Far fields: pattern symmetries
Far fields of transverse patterns with different symmetries. Left: hexagonal pattern consisting of three modes with higher harmonics, center: 'square' pattern where the corner modes are simultaneaously unstable modes and higher harmonics of the inner modes, right: competition of a square and a hexagonal pattern, both patterns share a common mode.
The fundamental process observable with a modulation instability is the initially explonential growth of a transverse modulation of the homogeneous pump beam from noise. The transverse spatial frequency of the growing mode is primarily determined by the spatial scale imposed through free space propagation to the feedback mirror and back. The azimutal orientation of the growing modes is initially undetermined, only nonlinear mode interaction leads to certain symmetries. In case that only modes with a single transverse wave number can grow, one always observed hexagonal patterns consisting of three modes with angles of 120 degrees in between [3]. If there are active modes with different wave numbers, mode interaction results in a quite different symmetries [4]. For the experimental system presented here such non-hexagonal modes are observed over a wide parameter region (multiplle pattern region[5]). Very often, more than a single pattern symmetry is a possible solution of the system, leading to effects such as coexistence and competition of patterns.
These properties mark the photorefractive single-feedback experiment as an attractive model system for the investigation of two-dimensional mode interaction in pattern formation. A high complexity of the observed patterns suggests research dealing with the phenomena of multistability and pattern competition. To this end, the investigation of static and dynamic control methods, primarily by means of amplitude and phase modulation in real and Fourier space, but also exploiting access to other parameters, is among the objectives of our research. The goal of the development of control methods is threefold: very often, simple suppression of undesired pattern formation is required. However, beyond mere suppression, control methods are sucessfully employed as tools for the analysis of pattern forming systems and, finally, self organized pattern formation is increasingly considered as a tool for the fabrication of structured materials [6],[7].

Experimental analysis

Experimental setup
Experimental setup (reduced to significant components). The optical diode serves to avoid direct destabilizing feedback into the frequency doubled Nd:YAG cw laser. The lens focusses the laser beam into the photorefractive Fe:KNbO3 crystal. By rotating the linear polarization using the half wave plate, one can select different electro-optic coefficients and thereby vary the photorefractive coupling (control parameter). The reflected beam exiting the crystal is observed and analyzed via a beam splitter. Finally, two lenses in the feedback arm image the external feedback mirror onto the crystal face or even into the crystal.
We investigate self-organized pattern formation in a single-mirror feedback experiment [8]. The first pump beam is directly obtained from the laser source and focused into the photorefractive crystal. The second beam is created by reflecting the original pump beam off the external mirror. Diffraction of the beam propagating to the mirror and back is responsible for the spatial coupling neccessary for the generation of transverse patterns.
Near and far field of a hexagonal pattern
Hexagonal pattern. Left: near field (crosssection of the beam leaving the crystal), right: far field (spatial Fourier transform)

Instead of placing the feedback mirror next to the photorefractive crystal, we project an external mirror using a 4f imaging setup. This fully equivalent variant is called virtual mirror [5] and allows for the virtual mirror to be placed within the nonlinear medium. This feature is crucial for accessing the experimentally highly interesting multiple pattern region that displays numerous pattern symmetries and phenomena such as multistability and pattern competition. Additionally, one obtains access to a Fourier plane in the center of the 4f setup. Thereby, we can modify the signal fed back into the nonlinear medium in amplitude and phase in Fourier space. This ability to change the feedback in the spatial frequency domain enables the use of control techniques virtually impossible in many non-optical pattern forming systems.

In most of the available parameter space, the system spontaneously generates hexagonal patterns, that consist of three modes with degenerate transverse wave numbers. For virtual mirror positions approximately in the center of the photorefractive crystal however, a variety of non-hexagonal patterns is observed in the multiple pattern region. The existence of several symmetries can be traced to the nonlinear interaction of modes with different wave numbers but roughly equal growth rates [9]. The source for the individual modes and the theoretical determination of their growth rates is a topic of current research.

Analytical modelling of the system

Numerical model of the photorefractive medium. Two counterpropagating pump beams are color-coded for visual separation. One observes a fully developed transverse modulation in both beams which leads to spatial separation of the beams' intensity maxima. The decreasing beam power towards the right is the result of the reflection at the induced distributed Bragg mirror.
Starting from the paraxial wave equation and the Kukhtarev model of the photorefractive effect, the system is modelled by three coupled partial differential equations[10],[11]. The first two equations describe the two counterpropagating wave envelope amplitudes (A1, A2), which are coupled via the induced Bragg mirror whose amplitude is Q.


The third equation captures the temporal development of the material change, i.e. the refractive index modulation, in dependence on the local intensity of the pump beams interference pattern. Boundary conditions providing one input beam on one side and the external feedback mirror on the other side of the crystal complete the model. This system of equations can now be treated with the tools of nonlinear physics, foremost a linear stability analysis, in order to compare predictions obtained by the model with experimental data. In addition, computer experiments can be pursued by numerically solving the equations, providing a bridge between experimental reality an simplifications of the model and checking for the model's limitations.